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Tailoring Lewis Acidity of Metal Oxides on Nickel to Boost . . . Neutral-pH water splitting for hydrogen production features a benign environment that could alleviate catalyst and electrolyzer corrosion but calls for the corresponding high-efficiency and earth-abundant hydrogen evolution reaction (HER) catalysts Herein, we first designed a series of metal oxides decorated on Ni as the model catalysts and found a volcano-shaped relationship between the
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Spin-State Effect of Tetrahedron-Coordinated Single-Atom Catalysts on . . . Spin state of active sites is one of the most influencing factors for the catalytic performance of electrocatalysts To date, most modulations are conducted on non-tetrahedrally coordinated metal sites, while tetrahedron-coordinated single-atom catalysts (TCSACs) have not been investigated yet This article presents a correlation between the spin state of TCSACs and their activities toward CO2